High efficiency second harmonic generation of nanojoule level femtosecond pulses

We demonstrate high efficiency second harmonic generation (SHG) of near infrared femtosecond pulses using a $\text{BiB}_{3}\text{O}_{6}$ crystal in a single-pass tight focusing geometry setup. A frequency doubling efficiency of $63\%$ is achieved, which is, to the best of our knowledge, the highest value ever reported in the femtosecond regime for such low energy (nJ-level) pumping pulses. Theoretical analyses of the pumping scheme focusing waist and the SHG efficiency are performed, by numerica